SNOM 2 (Gold particle probe)

It is well known that surface plasmon existing on a metal surface and a metal / dielectric interface causes strong field enhancement at the interface. According to the theoretical analysis, surface refractive index distribution mapping with a high contrast is predicted to be possible. A metal particle probe is considered to have the advantages of high experimental reproducibility, not requiring gap control, and not only the ability to obtain the surface image, but also to obtain the spectroscopic data of the sample. The scattering efficiency of a silver particle is higher than that of a gold particle, but the latter is more chemically stable. Therefore a gold particle is frequently used as a SNOM probe.

Sugiura et al. observed a dip on a cover glass and a gold colloidal particle adhering to the cover glass. However, these images were thought to have been an artifact problem due to the vertical displacement of the gold probe. On the other hand, the following are observed for a refractive index grating on a flat surface, which was made on a planar light waveguide circuit (PLC), by scanning an optically trapped 100-nm-diameter gold particle. The scattered Ar+ laser light from the gold particle has a high intensity due to the high refractive index of the grating with periods of 1.06 mm and 0.53 mm, both by s- and p-polarized illuminations.

Moreover, the surface profile of an optical disk tracking groove is also observed with and without the gold particle and the results compared to discuss the artificial effect due to the vertical displacement of the particle caused by the surface topology.

Experimental setup
Figure 1 shows an experimental setup to trap a gold particle with an upward-directed Nd:YAG laser beam (l = 1.06 mm) and to scan it on the sample surface two-dimensionally using an XY stage. The upward-directed laser beam has a higher trapping efficiency than the downward one. Figure 2(a) shows a photograph of the setup. The gold particle at the focal point of the objective lens is in the medium of a coverslip-shield chamber and is pushed onto the sample surface and scanned as shown in Fig. 2(b).

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Fig. 1. Experimental setup of SNOM using an optically trapped gold particle. A Nd:YAG laser is used for trapping, and an Ar+ laser is used for illuminating the gold particle. All the optical elements except mirrors to guide the lasers are installed inside the small optical box (white box in Fig. 5.22(a))for easy operation


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Fig. 2. Photograph of experimental setup of SNOM (a), and enlarged view of sample chamber (b)





An Ar+ laser (l = 488 nm) is focused through the same objective to illuminate the particle. The scattered light from the gold particle is collected through the objective and imaged on the pinhole (5 mm in diameter) in front of a PMT. The scattered light variation due to the interaction between the gold particle and the sample surface is recorded on a personal computer (PC). A CCD camera observes the operation of the gold particle in the medium. All the optical elements, except the mirrors to guide the Nd:YAG laser and Ar+ laser, are installed inside the optical box for easy operation.